Progress in Nano-Electro-Optics I

Basics and Theory of Near-Field Optics

By: Motoichi Ohtsu (Editor)

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Hardcover | 29 November 2002

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This volume focuses on fundamental aspects of nano-electro-optics. Starting with fiber probes and related devices for generating and detecting the optical near-field with high efficiency and resolution, the next chapter addresses the modulation of an electron beam by optical near-fields. Further topics include: fluorescence spectroscopy, in which sample molecules are excited by the evanescent surface plasmon field close to metallic surfaces; spatially resolved near-field photoluminescence spectroscopy of semiconductor quantum dots, which will become an essential issue in future electro-optical devices and systems; and, finally, the quantum theory of the optical near-field. This latter theory accounts for all the essential features of the interaction between optical near-fields and nanomaterials, atoms and molecules. Together these overviews will be a valuable resource for engineers and scientists working in the field of nano-electro-optics.

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"This unique monograph series entitled 'Progress in Nano-Electro-Optics' is being introduced to review the results of advanced studies in the field of electro-optics at nanometric scales and covers the most recent topics ... . this book is a very interesting one which can provide a very useful and multi-purpose tool for many users. ... Together these overviews will be a valuable resource for students, engineers and scientists. So let me recommend this book for everyone, readers or specialists ... ." (Yvon Renotte, Physicalia, Vol. 25 (4), 2003)

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High-Throughput Probes for Near-Field Optics and Their Applications	p. 1
High-Throughput Probes	p. 1
Mode Analysis in a Metallized Tapered Probe	p. 1
Light Propagation in a Tapered Probe with Ideal Metal Cladding	p. 4
Measurement of the Spatial Distribution of Optical Near-Field Intensity in the Tapered Probe	p. 6
Further Increase in Throughput	p. 10
Application to High-Density and High-Speed Optical Memory	p. 19
Using an Apertured Fiber Probe	p. 19
High-Density and High-Speed Recording Using a Pyramidal Silicon Probe on a Contact Slider	p. 20
Outlook	p. 27
References	p. 27
Modulation of an Electron Beam in Optical Near-Fields	p. 29
Introduction	p. 29
Review of Experiments	p. 30
Smith-Purcell Effect	p. 30
Schwarz-Hora Effect	p. 31
Basic Principle	p. 32
Microgap Interaction Circuits	p. 35
Circuit Configuration	p. 35
Transition Rates of Electrons	p. 36
Theoretical Analyses of a Microslit	p. 40
Near-Field Distributions	p. 40
Wave Number Spectrum	p. 43
Numerical Simulations	p. 44
Experiment	p. 47
Experimental Setup	p. 48
Electron Energy Spectrum	p. 48
Modulation with Laser Field	p. 51
Wave Number Spectrum	p. 52
Multiple-Gap Circuit	p. 53
Inverse Smith-Purcell Effect	p. 53
Experimental Setup	p. 55
Phase Matching Condition	p. 55
Field Distributions	p. 56
Microslit for Visible Light	p. 57
Conclusion	p. 59
References	p. 59
Fluorescence Spectroscopy with Surface Plasmon Excitation	p. 61
Introduction	p. 61
Theoretical Considerations	p. 61
Surface Plasmons at the Interface Between a (Noble) Metal and a Dielectric Medium	p. 61
Optical Excitation of Surface Plasmons	p. 64
Surface Plasmons for the Characterization of Thin Layers	p. 67
Electromagnetic Field Distribution near the Interface	p. 68
Fluorescent Chromophores near Metal Surfaces	p. 70
Experimental	p. 72
Results and Discussion	p. 74
Experimental Verifcation of Surface Field Enhancement	p. 74
Frontside Versus Backside Emission	p. 76
Conclusions	p. 80
References	p. 81
Optical Characterization of In(Ga)As/GaAs Self-assembled Quantum Dots Using Near-Field Spectroscopy	p. 83
Introduction	p. 83
Relaxation Mechanism	p. 84
Optical Properties of Self-assembled Quantum Dots: Far-Field Analysis	p. 86
Photoluminescence Spectroscopy	p. 86
Magneto-Optical Spectroscopy	p. 87
Photoluminescence Excitation Spectroscopy	p. 89
Raman Spectroscopy	p. 90
Near-Field Optical Spectroscopy	p. 92
Ground-State Emission	p. 94
Interaction with Phonons	p. 101
Carrier Relaxation	p. 106
Dephasing of Excited Carrier	p. 107
Spin Relaxation	p. 111
Conclusion	p. 115
References	p. 115
Quantum Theoretical Approach to Optical Near-Fields and Some Related Applications	p. 119
Introduction	p. 119
Basic Idea and Massive Virtual Photon Model	p. 120
Projection Operator Method	p. 121
Definition of the Projection Operator	p. 122
Properties of the Projection Operator	p. 122
Effective Operator and Effective Interaction	p. 123
Equation for the Operator J and Its Approximate Solution	p. 125
Effective Interaction Operator in an Approximation	p. 126
Electromagnetic Interaction with Matter: Minimal-Coupling and Multipole Hamiltonians	p. 127
Minimal-Coupling Hamiltonian	p. 127
Multipole Hamiltonian	p. 129
Elementary Excitation Modes and Electronic Polarization	p. 133
Polaritons and Electronic Polarization	p. 134
Optical Near-Field Interaction: Yukawa Potential	p. 137
Relevant Microscopic Subsystem and Irrelevant Macroscopic Subsystem	p. 137
P Space and Q Space	p. 138
Effective Interaction in the Nanometric Subsystem	p. 138
Effective Mass Approximation of Exciton Polaritons and Yukawa Potential	p. 141
Applications	p. 143
Single Atom Manipulation	p. 143
Fundamental Properties of Optical Near-Field Microscopy	p. 148
Outlook	p. 154
References	p. 155
Index	p. 159
Table of Contents provided by Syndetics. All Rights Reserved.

Progress in Nano-Electro-Optics I

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