Molecular Rydberg Dynamics

By: M. S. Child (Editor), The Royal Society

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Hardcover | 8 July 1999

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260 Pages

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27.94 x 20.32 x 2.54

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The study of molecular Rydberg states is a rapidly growing interdisciplinary field. This valuable report, constituting the proceedings of a Royal Society Discussion reflects the state of the present theoretical knowledge, and includes an introductory chapter for the non-specialist. e material is organised to bring out the wealth of observable effects. Some states commonly lead to competitive predissociation and autoionization, with relevance to atmospheric and astrophysical processes. Others, with higher angular momenta, have much longer lifetimes and high electronic degeneracies, which on one hand pose subtle problems for experimental interpretation, and on the other act as reservoirs for a class of remarkably stable so-called ZEKE states. New experiments to classify the formation mechanism of such states, and to exploit their properties, are described. The interplay between "quantum defect" and "ab initio" aspects of the theory is also underlined.

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Non-Fiction Science Physics Atomic & Molecular Physics Chemistry Physical Chemistry Quantum Physics & Quantum Mechanics & Quantum Field Theory Booktopia Publisher Services World Scientific Publishing

Preface
Frontispiece
The nature of molecular Rydberg states	p. 1
The Rydberg spectrum of ArH and KrH: calculation by R-matrix and generalized quantum defect theory	p. 17
Discussion	p. [s.n.]
Rydberg series of BaF: perturbation-facilitated studies of core-non-penetrating states	p. 43
Solved and unsolved problems of near-threshold spectroscopy of N[subscript 2] and CO	p. 63
Decay dynamics of hgh Rydberg states in atoms and molecules	p. 75
Discussion	p. 86
On the role of ions in pulsed field ionization zero-kinetic-energy photoelectron spectroscopy	p. 87
State-to-state dynamics in the high Rydberg states of polyatomic molecules	p. 105
Discussion	p. 118
Rotational propensities in the state selection of NH[subscript 3]+ by pulsed-field ionization	p. 121
Discussion	p. 143
Table of Contents provided by Blackwell. All Rights Reserved.

Molecular Rydberg Dynamics

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