| Preface | |
| Contributors | |
| Historical Introduction | |
| The Discovery of the Electron Spin | p. 1 |
| Preparing the Way for Paramagnetic Resonance | p. 13 |
| Paramagnetism, Before Magnetic Resonance | p. 25 |
| Cryomagnetism and Magnetic Resonance in Oxford Physics | p. 37 |
| The Scientific Work of E. K. Zavoisky | p. 45 |
| Spin-Lattice Relaxation Studies in Kazan University | p. 51 |
| Paramagnetic Resonance in the Early Years of the Zavoisky Institute | p. 57 |
| The First Sesquidecade of Paramagnetic Resonance | p. 63 |
| EPR in The Netherlands | p. 84 |
| EPR at Berkeley 1951-55: An Annotated Bibliography | p. 105 |
| EPR at Harvard | p. 111 |
| EPR: The Indian Scene | p. 132 |
| Transition Metals | |
| Hyperfine Structure | p. 150 |
| A Remembrance of ESR's Past | p. 161 |
| Lanthanides | p. 165 |
| High-spin Systems | p. 185 |
| Organic Radicals | |
| Early Studies of Exchange Between Paramagnetic and Diamagnetic Molecules | p. 196 |
| EPR and the History of the Thianthrene Cation Radical | p. 202 |
| Organic Radical Ions as Studied by EPR Spectroscopy | p. 213 |
| Theories of Molecular Electronic Structure | p. 236 |
| Spin Trapping | p. 241 |
| Gas Phase EPR | |
| Electron Paramagnetic Resonance in Gases | p. 265 |
| Early EPR in Some Gases | p. 271 |
| Electrochemically Generated Radicals | |
| EPR And Electrochemistry | p. 278 |
| Radicals Formed by Radiation | |
| Radicals I Have Loved: I - Organic Free Radicals | p. 295 |
| Radical Formation in Irradiated Biological Systems | p. 310 |
| EPR of Short-lived Radicals | p. 317 |
| Applications to Biological Systems | |
| Early Applications to Biological Systems | p. 331 |
| EPR of Metalloproteins: Truth Tables Revisited | p. 346 |
| In Vivo EPR | p. 361 |
| Biological Applications of EPR Involving Iron | p. 379 |
| Spin Labels | p. 410 |
| Site-Directed Spin Labeling: A Strategy for Determination of Structure and Dynamics of Proteins | p. 423 |
| EPR in Biochemistry | p. 436 |
| EPR Studies of Cells and Tissues | p. 451 |
| Spin-Spin Interactions | |
| Inhomogeneous Broadening, Spectral Diffusion, and All That | p. 460 |
| The Effect of Concentration and Oxygen in EPR | p. 469 |
| Electron Paramagnetic Resonance and the Phosphorescent State of Aromatic Organic Molecules | p. 482 |
| The Path that led to the Study of Luminescent Triplet States by EPR with Optical Detection in Zero Field | p. 496 |
| Triplet Exciton Spin Exchange Effects in the Ion Radical Salts of Tetracyanoquinodimethane | p. 512 |
| Electron-Electron Spin-Spin Splitting | p. 522 |
| EPR of Non-Kramers Systems in Biology | p. 530 |
| The Development of ENDOR and other Reminiscences of the 1950's | p. 548 |
| ENDOR in Liquids | p. 557 |
| ELDOR Spectroscopy | p. 577 |
| Chemically Induced Dynamic Electron Polarization (CIDEP) | p. 587 |
| RYDMR of Short-Lived Spin-Correlated Pairs | p. 602 |
| Time-Domain EPR | |
| Saturation Recovery | p. 607 |
| Electron Spin-Lattice Relaxation by Pulsed Field Sweep | p. 619 |
| Electron Spin Echo Experiments Then and Now | p. 629 |
| Electron Spin Echo in Siberia | p. 635 |
| Applications of Electron Spin Echo Modulation | p. 641 |
| Fourier Transform EPR | p. 652 |
| Linewidths, Lineshapes, and Spin-Relaxation in the One and Two-Dimensional ESR of Organic Radicals and Spin Labels | p. 658 |
| Imaging | |
| EPR Imaging | p. 684 |
| Development of EPR Instrumentation | |
| EPR at Varian: 1954-1974 | p. 695 |
| A Bruker EPR History | p. 717 |
| Very-High-Field EPR | p. 731 |
| Other EPR Detection Methods | |
| Multiquantum EPR | p. 741 |
| Longitudinal Techniques in ESR and ENDOR Spectroscopy | p. 758 |
| Microwave Amplitude Modulation and Short T[subscript 1] Measurement | p. 768 |
| From 10[superscript 10] Spins to a Single Spin | p. 781 |
| The Next 50 Years | p. 792 |
| Index | p. 794 |
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