Acidity and Basicity of Solids - Theory, Assessment and Utility : Proceedings of the NATO Advanced Study Institute, La Colle sur Loup (Nice), France, June 13-25, 1993

Proceedings of the NATO Advanced Study Institute, La Colle sur Loup (Nice), France, June 13-25, 1993

By: Jacques P. Fraissard (Editor), Leonidas Petrakis (Editor)

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Hardcover | 1 November 1994

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Historically, technological developments that have made use of the acidity/basicity of solids have often preceded an understanding of the phenomena involved. This, of course, is very expensive, and a far less efficient process than research based on a fundamental understanding of the science. For the last 50 years, therefore, a vast amount of research has been devoted to the subject: the rewards, in terms of technological advantage, were seen to be high. In the last few years, however, significant advances in the field have been achieved, in terms of our theoretical understanding, in instrumentation that allows research to be conducted in situ and under conditions appropriate to industrial processes, and in the realisation that a closer coupling between science and technology can improve our quest. It is against such a background that Acidity and Basicity of Solids presents the latest and best work in the field. For specialized workers in the field and university teachers of introductory as well as graduate courses. The more general reader will find the reviews particularly interesting.

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Preface
Historical Perspectives of Acidity and Basicity. Part 1: 4000 B.C.-1800 A.D.	p. 1
Historical Perspectives of Acidity and Basicity. Part 2: 1800 A.D.	p. 13
Theory of Acids and Bases. I. Relationships between Structure and Acidity and Basicity. II. Theory of Medium Effects on Acidity and Basicity	p. 33
Quantum Mechanical Study of Acid Base Reactions in the Solid State	p. 53
Acidity and Basicity Concepts: The Density Functional Viewpoint Based on an Atoms-in-Molecules Sensitivity Analysis - a Tutorial	p. 95
The Acid Function in Zeolites	p. 127
Basicity in Zeolites	p. 181
The Nature of Lewis Acid Sites of Aluminium Oxide and in Zeolites as Studied by IR Spectra of Adsorbed Hydrogen	p. 199
Structure and Composition Factors in the Acidity and Basicity of Inorganic Molecular Metal-Oxygen Cluster Catalysts and Their Influence on the Surface and Catalytic Properties	p. 217
The Acidity and Basicity of Solids: Intrinsic Properties of the surface, Its Structure and Composition	p. 237
Characterization of Bronsted and Lewis Acidity by Nuclear Magnetic Resonance Spectroscopy	p. 255
Characterization of Bronsted Acidity of Solids by Rigid-Lattice Broad-Line [superscript 1]H-NMR. Part 1: Methodology	p. 279
Comparison of Different Zeolites Studied by two Proton NMR Techniques: Broad-Line at 4 K and High Resolution Mas at 300 K	p. 291
Catalytic Chemistry of Perfluorinated Resinsulfonic Acids: Reactions, Mechanistic Aspects and Superelectrophilic Activation	p. 305
The Mechanism of Proton Transfer and the Nature of Protonated Intermediates in Heterogeneous Acid Catalysis	p. 335
Acid-Base Bifunctional Catalysis	p. 353
Generation of Acidity (Amount and Strength) in Silicoaluminophosphates (SAPO Zeolites). Examples of SAPO-5, -11, -34 and -37	p. 375
Determination of Silicon Coordination Spheres in SAPO-37 Molecular Sieve with MS-EXCEL	p. 391
Importance of Preparation of Acidic and Basic Solid Materials	p. 403
Regulation of Surface Acidity of Oxidic Carriers used for the Preparation of Supported Catalysts	p. 415
Industrial Catalytic Applications of Acidic Molecular Sieves	p. 445
Application of Solid Acids and Bases to Various Fields	p. 475
Characterization of Bronsted Acidity of Solids by Rigid-Lattice Broad-Line [superscript 1]H-NMR. Part 2: Applications	p. 485
Closing Remarks	p. 501
Index	p. 503
Table of Contents provided by Blackwell. All Rights Reserved.

Acidity and Basicity of Solids - Theory, Assessment and Utility : Proceedings of the NATO Advanced Study Institute, La Colle sur Loup (Nice), France, June 13-25, 1993

Proceedings of the NATO Advanced Study Institute, La Colle sur Loup (Nice), France, June 13-25, 1993

At a Glance

Hardcover

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